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Positive Matrix Factorization (PMF) receptor modeling

In order to identify the sources of aerosols in the western United States, Positive Matrix Factorization (PMF) receptor model is applied to the 24-hr integrated aerosol chemical composition data obtained at the Class I areas of the Western Regional Air Partnership (WRAP) region through the Interagency Monitoring of Protected Visual Environments (IMPROVE) program. The IMPROVE sites in the WRAP region are grouped into 18 sub-regions (including West Texas region) as shown in Figure 1. PMF is applied to each group to generate profiles of source factors. Normalized source profiles and the quantitative source contributions for each resolved factor are calculated. The major sources that contribute to the aerosol loadings in the western United States are identified. The similarities and differences of chemical source profiles, and the major aerosol source contributors in different regions of the western United States are investigated. Based on the profile and the daily contribution to aerosol concentration of each source factor, the contributions of source factors to the aerosol light extinction coefficients are estimated using the IMPROVE method. The importance of the major aerosol sources to regional haze and visibility in the Class I areas of the western United States is discussed.

 

Figure 1. Grouping of Class I areas.

 

PMF Modeling Results (All Sampling Days)

Alaska

California Coast

Central Rockies

Colorado Plateau

Columbia River Gorge

Death Valley

Great Basin

Hells Canyon

Hawaii

Mogollon Plateau

Northern Great Plains

Northern Rockies

Northwest

Oregon and Northern CA

Sierra Nevada

Southern Arizona

Southern California

West Texas

PMF Modeling Results (20% Worst Visibility Days)

Alaska

California Coast

Central Rockies

Colorado Plateau

Columbia River Gorge

Death Valley

Great Basin

Hells Canyon

Hawaii

Mogollon Plateau

Northern Great Plains

Northern Rockies

Northwest

Oregon and Northern CA

Sierra Nevada

Southern Arizona

Southern California

West Texas